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Strong coupling in light-matter interaction with THz metamaterials and microcavity

목차

I. Introduction 1
1. Strong coupling in light-matter interaction 1
2. Organization of the thesis 9
3. Reference 12
II. Background 14
1. THz time-domain spectroscopy and imaging technology 14
2. Lead halide perovskite (MAPbI3) 19
3. Metamaterials 24
4. Fabry-Perot cavity 39
5. References 44
III. Phonon-Polaritons in Lead Halide Perovskite Film Hybridized with THz Metamaterials 62
1. Introduction 62
2. Observation of Phonon polariton using THz metamaterials 64
3. Dispersion curve 69
4. Calculation of strong coupling 74
5. In situ phonon-polariton formation 77
6. Methods 83
7. Conclusion 84
8. References 86
IV. Mechanical control of quantum states in lead halide perovskite phonons strongly coupled in THz microcavity 95
1. Introduction 95
2. Observation of Phonon polariton using THz Fabry-Perot Cavity 97
3. Dispersion curve 104
4. Calculation of strong coupling 108
5. Flexible phonon-polariton device 112
6. Methods 117
7. Conclusion 118
8. References 119
V. Conclusion 203

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